All Positions

Research
Optical physics

Thin film lithium niobate nonlinear photonics

DC-15
ECL and RMIT
Ecully (FR) and Melbourne (AU)

Host organizations

Proposed Projects

Option 1

Efficient nonlinear broadband supercontinuum light sources in strip-loaded LNOI

Despite the high application potential of nonlinear optics for all-optical information processing, no nonlinear material candidate has emerged as a clear choice to complement silicon photonics so far. On the one hand, wide band gap semiconductors have been investigated, but their integration onto silicon photonics is not straightforward. Glass materials have also been explored, but their relatively weak nonlinearity precludes the realization of compact devices. Lithium niobate (LiNBO3) possesses both a second-order (c(2)) and third-order (c(3)) nonlinearity, which proves useful for both electro-optical modulation and also all-optical signal processing devices. Recently, thin-film lithium niobate on insulator wafers have become commercially available and emerged as a highly promising platform for integrated nonlinear optics. Most importantly, this platform supports tightly confining waveguide geometries, a boost for nonlinearities, while additionally opening opportunities for dispersion engineering, which is key to device efficiency and broadband processes, such as supercontinuum. In this context, RMIT has developed a complementary route towards high performance thin-film lithium niobate based devices that exploits strip loading of another thin film, silicon nitride (Si3N4) for instance, which is patterned instead of the lithium niobate so as to support low loss guided modes. This approach elegantly alleviates the need for lithium niobate patterning, while still offering relatively tightly confining geometries (Aeff ~2µm2) and the possibility to engineer the dispersion which is key for broadband supercontinuum.

The aim of this project will be to push this approach for broadband supercontinuum generation that can reach out to the mid-IR band (5um), where many molecules of importance for the defense and environment have strong absorption fingerprint. Part of the strategy will involve quasi phase matching with periodic poling of lithium niobate to increase the efficiency of difference frequency generation processes pumped at telecom wavelengths. This will be also used as a means to increase cascaded c(2) processes and further promote spectral broadening of the pump.

A.Boes et al., Lithium niobate photonics: Unlocking the electromagnetic spectrum.Science379,eabj4396(2023).DOI:10.1126/science.abj4396
Roy, A., Ledezma, L., Costa, L. et al. Visible-to-mid-IR tunable frequency comb in nanophotonics. Nat Commun 14, 6549 (2023). https://doi.org/10.1038/s41467-023-42289-0
C. Wang, et al. Integrated lithium niobate electro-optic modulators operating at CMOS-compatible voltages, Nature 562, 101 (2018). https://doi.org/10.1038/s41586-018-0551-y
M. Zhang et al. Broadband electro-optic frequency comb generation in a lithium niobate microring resonator, Nature 568, 373 (2019). https://doi.org/10.1038/s41586-019-1008-7
M. Jankowski et al. Ultrabroadband nonlinear optics in nanophotonic periodically poled lithium niobate waveguides, Optica 7, 40 (2020).
Y. Okawachi et al. Chip-based self-referencing using integrated lithium niobate waveguides, Optica 7, 702 (2020).
D. Zhu et al. Integrated photonics on thin-film lithium niobate, Adv. Opt. Photon. 13, 242 (2021).

Option 2

Efficient nonlinear integrated microcombs in thin film LNOI

Despite the high application potential of nonlinear optics for all-optical information processing, no nonlinear material candidate has emerged as a clear choice to complement silicon photonics so far. On the one hand, wide band gap semiconductors have been investigated, but their integration onto silicon photonics is not straightforward. Glass materials have also been explored, but their relatively weak nonlinearity precludes the realization of compact devices. Lithium niobate (LiNBO3) possesses both a second-order (c(2)) and third-order (c(3)) nonlinearity, which proves useful for both electro-optical modulation and also all-optical signal processing devices. Recently, thin-film lithium niobate on insulator wafers have become commercially available and emerged as a highly promising platform for integrated nonlinear optics. Most importantly, this platform supports tightly confining waveguide geometries, a boost for nonlinearities, while additionally opening opportunities for dispersion engineering, which is key to device efficiency and broadband processes, such as optical frequency combs. The combination of both c(2)and c(3) responses can, in contrast with silicon where only c(3) does exist, provide new ways of electrically tuning all-optical nonlinear functions. Furthermore, the birefringence of lithium niobate and ferroelectric domain inversion capabilities provide opportunities for phase matching and quasi phase matching, which is critical for frequency conversion processes, such as four-wave mixing or high-order harmonic generation.

The specific objectives of this PhD study will be (1) to exploit strip-loaded lithium niobate on insulator resonators to design and realize highly efficient c(3) nonlinear devices with anomalous dispersion for comb generation, (2) to experimentally demonstrate the integration of electro-optical modulators with c(3) ring resonators on a single chip, where the modulation frequency of the modulator can be tuned to match the free spectral range of the ring resonator, which will enable the efficient generation of optical frequency combs, (3) explore the alternative path offered by c(2) nonlinear optics via quasi-phase matching in lithium niobate for the generation of optical frequency combs and (4) use the c(2) response of lithium niobate to realize tunable nonlinear functions.

A.Boes et al., Lithium niobate photonics: Unlocking the electromagnetic spectrum.Science379,eabj4396(2023).DOI:10.1126/science.abj4396
Roy, A., Ledezma, L., Costa, L. et al. Visible-to-mid-IR tunable frequency comb in nanophotonics. Nat Commun 14, 6549 (2023). https://doi.org/10.1038/s41467-023-42289-0
C. Wang, et al. Integrated lithium niobate electro-optic modulators operating at CMOS-compatible voltages, Nature 562, 101 (2018). https://doi.org/10.1038/s41586-018-0551-y
M. Zhang et al. Broadband electro-optic frequency comb generation in a lithium niobate microring resonator, Nature 568, 373 (2019). https://doi.org/10.1038/s41586-019-1008-7
M. Jankowski et al. Ultrabroadband nonlinear optics in nanophotonic periodically poled lithium niobate waveguides, Optica 7, 40 (2020).
Y. Okawachi et al. Chip-based self-referencing using integrated lithium niobate waveguides, Optica 7, 702 (2020).
D. Zhu et al. Integrated photonics on thin-film lithium niobate, Adv. Opt. Photon. 13, 242 (2021).

Option 3

Ultra-high Q factor lithium niobate resonators for mid-IR Kerr combs

Despite the high application potential of nonlinear optics for all-optical information processing, no nonlinear material candidate has emerged as a clear choice to complement silicon photonics so far. On the one hand, wide band gap semiconductors have been investigated, but their integration onto silicon photonics is not straightforward. Glass materials have also been explored, but their relatively weak nonlinearity precludes the realization of compact devices. Lithium niobate (LiNBO3) possesses both a second-order (c(2)) and third-order (c(3)) nonlinearity, which proves useful for both electro-optical modulation and also all-optical signal processing devices [1]. Recently, thin-film lithium niobate on insulator wafers [2] have become commercially available and emerged as a highly promising platform for integrated nonlinear optics [3]. Most importantly, this platform supports tightly confining waveguide geometries, a boost for nonlinearities, while additionally opening opportunities for dispersion engineering, which is key to device efficiency and broadband processes, such as optical frequency combs [4,5]. In this context, RMIT has developed a complementary route towards high performance thin-film lithium niobate based devices that exploits strip loading of another thin film, silicon nitride (Si3N4) for instance, which is patterned instead of the lithium niobate so as to support low loss guided modes. This approach elegantly alleviates the need for lithium niobate patterning, while still offering relatively tightly confining geometries (Aeff ~2µm2) and the possibility to engineer the dispersion which is key for the generation of frequency combs.

While much has been done with the lithium niobate on insulator (LNOI) platform in the telecom band, this material is transparent up to the mid-IR and could support low loss modes up to about 5um, reaching out the spectral window where many biomolecules of importance for defence and environmental applications have strong molecular fingerprints. The aim of this PhD will be to design and fabricate high quality factor microresonators (microrings, microdisks or photonic crystal cavities) that can support low loss confined modes at these long wavelengths. These will be specifically engineered, using for instance photonic molecules consisting of coupled cavities, and adequate coupling strategies (e.g. using pulley waveguides) will be deployed to sustain optical Kerr microcombs in the mid-IR.

A.Boes et al., Lithium niobate photonics: Unlocking the electromagnetic spectrum.Science379,eabj4396(2023).DOI:10.1126/science.abj4396
Roy, A., Ledezma, L., Costa, L. et al. Visible-to-mid-IR tunable frequency comb in nanophotonics. Nat Commun 14, 6549 (2023). https://doi.org/10.1038/s41467-023-42289-0
C. Wang, et al. Integrated lithium niobate electro-optic modulators operating at CMOS-compatible voltages, Nature 562, 101 (2018). https://doi.org/10.1038/s41586-018-0551-y
M. Zhang et al. Broadband electro-optic frequency comb generation in a lithium niobate microring resonator, Nature 568, 373 (2019). https://doi.org/10.1038/s41586-019-1008-7
M. Jankowski et al. Ultrabroadband nonlinear optics in nanophotonic periodically poled lithium niobate waveguides, Optica 7, 40 (2020).
Y. Okawachi et al. Chip-based self-referencing using integrated lithium niobate waveguides, Optica 7, 702 (2020).
D. Zhu et al. Integrated photonics on thin-film lithium niobate, Adv. Opt. Photon. 13, 242 (2021)

Supervisors

Research Areas

Physics, Photonics, Nonlinear Optics